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You will see the Delete or Unsubscribe option when clicking on a recipient either via a Global Search or from with a Group or List. (See above notes for definitions.)
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To Remove recipient from
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As seen above, click the Modify option, click the Assign recipients to group tab. You can remove the recipient from any group(s) by unchecking the adjacent box.
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groups
Click the View profile option and then click on the Groups tab. To change assignments, click "Manage group assignment".